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Abstract

We report rare examples of exclusive benzylic C–H oxidative addition in industrially important methylarenes using simple η⁴-arene iridium complexes. Mechanistic studies showed that coordinatively unsaturated η²-arene intermediates are responsible for the selective activation of benzylic, not aromatic C–H bonds and formation of stable benzyl complexes after trapping with a phosphine ligand.

This article is Open Access

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Article information

DOI

https://doi.org/10.1039/D1CC03445F

Article type

Communication

Submitted

28 Jun 2021

Accepted

13 Jul 2021

First published

13 Jul 2021

This article is Open Access

Chem. Commun., 2021,57, 7894-7897

Selective, radical-free activation of benzylic C–H bonds in methylarenes

A. P. Y. Chan, M. Jakoobi, C. Wang, Y. Tian, N. Halcovitch, R. Boulatov and A. G. Sergeev, Chem. Commun., 2021, 57, 7894 DOI: 10.1039/D1CC03445F

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Downtown Sounds

Downtown Sounds started as a small gathering hosted in an alley, turning the underutilized space into something extraordinary. And extraordinary it became. With each year the event grew, now taking up two entire city blocks on Bay and Prospect Streets. Downtown Sounds draws bands from across the country and folks from Whatcom County and beyond to share in their love of music. After 17 years of this beloved, award-winning, urban music festival, it is firmly cemented as Downtown Bellingham's hottest summer attraction.

2021 Series Lineup and Schedule:

August 4:Nite Wave with Analog Brass
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August 18:High Step Society with Stephanie Anne Johnson & The Hidogs
August 25: The Dusty 45s with Nuages

Beer garden opens at 5:30pm. Music from 6:00-9:00pm. Back on Bay & Prospect Streets.

Community Health & Safety

After June 30, 2021 physical distancing and capacity limitation restrictions were lifted for outdoor events. However, due to growing concern regarding the Delta variant, we have a few guidelines for Downtown Sounds concerts.

Guidelines:

• Please stay home if you are sick, or if you’ve been in contact with someone who is sick.

• Face coverings are required for any concert attendees who are unvaccinated, and all attendees are encouraged to bring a mask.

• Whatcom County Health Department recommends individuals wear a mask or face covering during crowded outdoor events, like Downtown Sounds

Ultimately, getting vaccinated and wearing a mask is the best way to help keep our community healthy. Please be considerate of others while enjoying Downtown Sounds, and thank you for continuing to keep each other safe!

Holly Street closure:

To allow for more space among concert goers, we’ll be closing Holly Street to through traffic on Wednesdays in August so that we can all enjoy the music with a little more space to spread out.

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